1. Kuroshitsuji / Black Butler
2. Axis Powers Hetalia
3. Elfen Lied
4. Jigoku Shoujo
5. Lucky Star
With some honorable mentions going to Mnemosyne no Musume Tachi, FMA, and Sayonara Zetsubo Sensei.
As for movies (they get their own category in my book):
1. Tokyo Godfathers (Satoshi Kon)
2. Paprika (Satoshi Kon)
3. The Girl Who Leapt Through Time
4. Spirited Away
5. Grave of the Fireflies
I don't have them in an order but
1)Baccano!(Why have i yet to see this mentioned?)
2)Lucky Star
3)Shaman King(the manga... so far its pretty good)
4)Death Note
5)Darker than Black
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